Lee, K. F.; Villeneuve, D. M.; Corkum, P. B.; Stolow, A. and Underwood, J. G.
|DOI (Digital Object Identifier) Link:||http://doi.org/10.1103/PhysRevLett.97.173001|
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We experimentally demonstrate field-free, three-dimensional alignment (FF3DA) of polyatomic asymmetric top molecules. We achieve FF3DA in sulfur dioxide gas using two time-delayed, orthogonally polarized, nonresonant, femtosecond laser pulses. Our method avoids the use of rotational revivals and is therefore more robust to temperature. The alignment is probed using time-delayed coincidence Coulomb explosion imaging. FF3DA will be important for all molecular imaging, dynamics, or spectroscopy experiments for which random alignment leads to a loss of information.
|Item Type:||Journal Article|
|Academic Unit/Department:||Faculty of Science, Technology, Engineering and Mathematics (STEM) > Physical Sciences
Faculty of Science, Technology, Engineering and Mathematics (STEM)
|Depositing User:||Users 8955 not found.|
|Date Deposited:||05 May 2009 13:36|
|Last Modified:||02 Aug 2016 13:25|
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